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I have noticed that enchanted bone fragments sell very high and I assume, therefore, they are rare.
No all the collection items are random items, any one has the same chance of being anything else. The only place I have noticed is not is the WC there u seem to get orc bones 99.9% of the time :P
I do know that some can only be gotten in certain zones or even spots in zones. The leaf collection is one, if you got to druid rings in commonlands there is one spawn there that gives a leaf more then anything else. So all you have to do is find out where the spawn is and go get your own, thats what I have done. And befoer some says it no I have not collected all 300+ collections in the game but have done 150+ of them.
The reason I know this is true is that the bones your are looking for are in commonlands also. I myself need 2 Glowing shards hehehe and they go for high price on our server well untill I find where they spawn and flood the market with em :)